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To this end, the BCP micelles under illumination should undergo a photoreaction that shifts the hydrophilic hydrophobic balance to make the micelles structurally or morphologically unstable in aqueous solution With azobenzene-containing amphiphilic BCPs, the photoreaction concerned is the reversible trans cis photoisomerization of the chromophore upon UV and visible light illumination, respectively From both the design and synthetic considerations, it is better to link azobenzene moieties onto the hydrophobic polymer In this case, as schematically illustrated in Fig 61, the hydrophobic block, bearing pendant azobenzene moieties in the more stable trans isomer can form the hydrophobic core of the core shell micelle or the membrane of the vesicle.

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bimolecular layer (bilayer) of phospholipids, with their long alkyl chains oriented inwards (Fig. 6.9). Electron microscope studies have revealed that the central layer corresponds to this largely hydrocarbon region. In fact, biological membranes are still more complex as will be discussed in Section 6.4.2.

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Although the official introduction of blade servers did not come until 2001, early versions of a PC on a card actually existed several years prior to that. Before the Internet explosion and broadband access, the early bulletin board operators were beginning to morph into the first Internet service providers (ISPs). These companies needed lots of servers to support sessions for their dial-up customers, and standard tower or rack-mount servers just took up too much space. Many enterprises were also supporting remote workforces using remote access/control software, such as Carbon Copy or PC Anywhere, for employees or partners to access in-house network resources from a remote PC or terminal.

6.4.1 Composition of biological membranes Biological membranes consist of lipids, proteins and also sugars, sometimes mutually bonded in the form of lipoproteins, glycolipids and glycoproteins. They are highly hydrated water forms up to 25 per cent of the dry weight of the membrane. The content of the various protein and lipid components varies with the type of biological membrane. Thus, in

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for the encapsulation of hydrophobic and hydrophilic agents, respectively (polymer vesicles can also load hydrophobic agents in the membrane, which is not depicted in Fig. 6.1). Upon illumination with UV light, azobenzene moieties can be converted to the cis isomer. To shift the hydrophilic hydrophobic balance towards the destabilization (dissociation) of the micelles, obviously the cis isomer of azobenzene must be signi cantly more polar than the trans isomer. This is possible by appropriate choice of substitutions on azobenzene. A hint comes from azobenzene without substitution, for which it is known that the elongated trans form has a zero dipole moment, while the bent cis form has a dipole moment of B3 D (Kumar and Neckers, 1989). To obtain a small (near zero) dipole moment for trans-azobenzene linked to the polymer chain backbone, the use of the same substitution groups on the para positions of azobenzene would be most useful since this substitution pattern gives a nearly symmetrical structure for the trans isomer, with no separation of positive and negative charge centers. On the other hand, the cis isomer should have an increased dipole moment owing to the conformational (shape) change. On the contrary, azobenzene structures with strong electron-donor and electron-acceptor groups on the para positions, which would have a higher dipole

Several companies (Cubix, ChatCom, and CommVision) saw some initial success in this market niche in the mid 1990s, delivering PC-on-a-card servers that resided in a common chassis. By 1997, however, Citrix Systems had achieved dominance in the remote access/control marketplace, displacing the Carbon Copy dedicated-PC approach. Citrix s software, somewhat similar to virtualization software, served up multiple PC sessions from a single server to multiple remote PCs acting as terminals. Since Citrix charged a per-server license fee, not a per-PC user license fee, it was much cheaper for users to implement, and by 2000 the success of Citrix had changed the market and closed the window for these early PC bladelike entrants.

Fig. 6.8 Electron photomicrograph of mouse kidney mitochondria. The structure of both the cytoplasmatic membrane (centre) and the mitochondrial membranes is visible on the ultrathin section. Magnification 70,000x. (By courtesy of J. Ludvik)

0.01 0 200 400 600 800 Relaxation time (s) 1000 1200

Fig. 6.9 Characteristic structures of biological membranes. (A) The fluid mosaic model (S. J. Singer and G. L. Nicholson) where the phospholipid component is predominant. (B) The mitochondrial membrane where the proteins prevail over the phospholipids

Figure 7.10. The effect of light on the dynamic properties of physical cross-links between azobenzene-modi ed poly(acrylate) and poly(cyclodextrin). The relaxation modulus in stress relaxation experiments is plotted after application at time zero of a xed strain to a 0.7% polymer solution in water (polymer structure, cf. Fig. 7.1, with n = 11 and x = 3) with polycyclodextrin at 0.25% (lower curves) or 0.5% (higher moduli). The sample was either incubated for 24 h in the dark (dark-adapted, closed symbols) or continuously exposed to UV before and after loading in the rheometer (open symbols). Details on the samples composition are given in Pouliquen et al. (2007).

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