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397 interesting example is a cell with two different chlorophyll-based absorbers The cathodic process starts by photoexcitation of a modified natural chloroplast with deactivated photosystem II (PS II for terminology of photosynthetic processes see page 469) The remaining PS I reduces, for example, anthraquinone-2-sulphonate The regenerative cycle of PS I is linked to tetramethyl-p-phenylenediamine which is cycled at the cathode The complementary anodic process is O2 evolution by the action of a second chloroplast system with active PS II; electrons from photoexcited PS II are transferred to the tetramethyl-p-phenylenediamine and the cycle is terminated by its oxidation at the anode The whole cell resembles photosynthesis, the net output being O2 and reduced anthraquinone-2-sulphonate (cf Section 652) The efficiency of the photocurrent generation in practical photogalvanic cells is generally low, since it is limited by short lifetimes of the excited dyes, parasitic electron transfer reactions, etc.

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Anisotropic bending and unbending behavior of azobenzene liquid crystalline gels by light exposure Adv Mater 15(3):201 205 Ishow E, et al 2006 Structural and photoisomerization cross studies of polar photo chromic monomeric glasses forming surface relief gratings Chem Mater 18(5):1261 1267 Jager C, Bieringer T, Zilker SJ 2001 Bicolor surface reliefs in azobenzene side chain polymers Appl Opt 40(11):1776 1778 Jiang XL, Kumar J, Kim DY, Shivshankar V, Tripathy SK 1996 Polarization dependent recordings of surface relief gratings on azobenzene containing polymer lms Appl Phys Lett 68(19):2618 2620 Jiang XL, Li L, Kumar J, Kim DY, Tripathy SK 1998 Unusual polarization dependent optical erasure of surface relief gratings on azobenzene polymer lms Appl Phys Lett 72(20):2502 2504 Kameda M, Sumaru K, Kanamori T, Shinbo T 2003 Photoresponse gas permeability of azobenzene functionalized glassy polymer lms J Appl Polym Sci 88(8):2068 2072 Kaneko F, et al 2002.

The importance of the photogalvanic effect rests in basic electrochemical research of homogeneous photoredox reactions To this purpose, original experimental techniques have been developed, eg voltammetry with an optically transparent rotating disk electrode The photoexcitation of reactants makes the study of redox reactions possible in a considerably broader region of the Gibbs free energy changes than with the ground-state reactants This brings interesting conclusions, for example, for the formulation of a more general theory of electron transfer, preparation of compounds in less-common oxidation states, etc 5104 Semiconductor photoelectrochemistry and photovoltaic effects Basic properties of semiconductors and phenomena occurring at the semiconductor/electrolyte interface in the dark have already been discussed in Sections 241 and 451 The crucial effect after immersing the semiconductor electrode into an electrolyte solution is the equilibration of electrochemical potentials of electrons in both phases.

In order to quantify the dark- and photoeffects at the semiconductor/electrolyte interface, a common reference level of electron energies in both phases has to be defined Let us choose, as an arbitrary reference level, the energy of an electron at rest in vacuum, e0 (cf Section 312) This reference energy is obvious in studies of the solid phase, but for the liquid phase, the Trasatti's conception of 'absolute electrode potentials' (Section 315) has to be adopted The formal energy levels of the electrolyte redox systems, REDOX, referred to (), are given by the relationship:.

Photo induced fabrication of surface relief gratings in alternate self assembled lms containing azo dye and alignments of LC molecules Coll Surf A 198:805 810 Kawatsuki N, Uchida E, Ono H 2003 Formation of pure polarization gratings in 4 methoxyazobenzene containing polymer lms using off resonant laser light Appl Phys Lett 83(22):4544 4546 Keum CD, Ikawa T, Tsuchimori M, Watanabe O 2003 Photodeformation behavior of photodynamic polymers bearing azobenzene moieties in their main and/or side chain Macromolecules 36(13):4916 4923 Kim DY, et al 1995a Polarized laser induced holographic surface relief gratings on polymer lms Macromolecules 28(26):8835 8839 Kim DY, Tripathy SK, Li L, Kumar J 1995b Laser induced holographic surface relief gratings on nonlinear optical polymer lms Appl Phys Lett 66(10):1166 1168 Kim DY, et al 1997 Photo fabrication of surface relief gratings on polymer lms Macromol Symp 116:127 134 Kim M H, Kim J D, Fukuda T, Matsuda H.

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2000 Alignment control of liquid crystals on surface relief gratings Liq Cryst 27(12):1633 1640..

where R E DOX is the standard redox potential of the particular redox system and cox, cred the concentrations of the oxidized and reduced forms,

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