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K , cr, Br, r, o r , NO 2 -, NO 3 OH~, F " , CNS", NCO~, H S " , C1O 3 ", C1O 4 ", BrO 3 ~, IO 4 ", MnO 4 ", HCOCT, citrate", CH 3 NH 3 + Hg 2 2+ , SO 4 2 -, S 2 O 3 2 ", S 2 O 6 2 ", S 2 O 8 2 ", Se 4 2 ", CrO 4 2 ~, HPO 4 2 ~, PO 4 3 ~, Fe(CN) 6 3 ~, Cr(NH 3 ) 6 3+ , Co(NH 3 ) 6 3+ , Co(NH 3 ) 5 H 2 O 3+ , NH 3 + CH 2 COOH, C 2 H 5 NH 3 + N a \ CdCl + , C1O2", IO 3 ", HCO 3 ", H 2 PO 4 ~, H S ( V , H 2 AsO 4 -, Pb 2 + , CO 3 2 ", SO 3 2 ", MoO 4 2 ", Co(NH 3 ) 5 Cl 2+ , Fe(CN) 6 NO 2 ", CH 3 COO", CH 2 C1COCT, (CH 3 ) 4 N + , (C 2 H 5 ) 2 NH 2 + , NH 2 CH 2 COO" Sr 2+ , Ba 2 + , Ra 2 + , Cd 2+ , Hg 2 + , S2~, S 2 O 4 2 ", WO 4 2 ", Fe(CN) 6 4 -, CHC1 2 COO~, CC1 3 COO + , (C 2 H 5 ) 3 NH + , C 3 H 7 NH 3 + Li + , Ca 2+ , Cu 2 + , Zn 2 + , Sn 2+ , Mn 2 + , Fe 2 + , Ni 2 + , Co 2 + , Co(ethylendiamine) 3 3+ , C 6 H 5 COO', C 6 H 4 OHCOCT, (C 2 H 5 ) 4 N + , (C 3 H 7 ) 2 NH 2 + Mg 2+ , Be 2+ H + , Al 3 + , Fe 3 + , Cr 3+ , Sc 3+ , La 3 + , In 3 + , Ce 3 + , Pr 3+ , Nd 3 + , Sm 3+ Th 4 + , Zr 4 + , Ce 4 + , Sn 4+.

An elegant anisotropic translation mechanism was developed by Le n, Fiorini, and Nunzi (Le n et al., 1998a,b). In this model, material transport occurs essentially because of an (orientational) concentration gradient. It is suggested that the rapid cycling of chromophores between trans and cis states enables transient, random motion of molecules preferentially along their long axis, because of the inherent anisotropy of azo molecules. The probability of undergoing a random-walk step is proportional to the probability of isomerization, which of course depends on the light intensity and the angle between the chromophore dipole and the incident electric vector. This predicts a net ux of molecules out of the illuminated areas and into the dark regions, consistent with experiment. This process would be enhanced by pointing dipoles in the direction of the light gradient (toward the dark regions). This would appear to explain the polarization dependence to a certain extent. In contrast to experiment, however, this model implies the best results when using small molecules, not polymers. For polymer chains laden with many chromophores, random motion of these moeities would presumably lead to a tug-of-war that would defeat net transport of the chain. It is at present not clear that the driving force in this model is suf cient to account for the substantial mass transport (well below Tg) observed in experiments.

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Mechanisms based on electromagnetic forces are promising since they naturally include the intensity and polarization state of the incident light eld. In the mean eld model developed by Pedersen and coworkers (Pedersen et al., 1998; Pedersen and Johansen, 1997), each chromophore is subject to a potential resulting from all the other chromophore dipoles in the material. Irradiation orients chromophores, and this net orientation leads to a potential that naturally aligns other chromophores. Furthermore, there is an attractive force between side-by-side chromophores that are aligned similarly. This leads to a net force on chromophores in illuminated areas, causing them to order and aggregate. Obviously this model predicts an accumulation of chromophores in the illuminated areas. Thus surface relief peaks will be aligned with light intensity maxima. Although this result does not agree with experiments in amorphous samples, it is consistent with many experiments on LC systems. The mean- eld model inherently includes intermolecular cooperativity and orientational order, and it appears natural that it would be manifest in mobile LC systems. The polarization state of incident light is

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