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yielding the usual form of the equation for the activity coefficient (cf. p. 11): log y* =-,4z 2 VZ (1.3.24)

4:5

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termed the Debye-Hilckel limiting law. Coefficient A has the numerical value A = 5.77057 x 10 4 (Dr)" 3/2 = 1.82481 x 10\DT)-3/2 and, for water at 25 C, A = 1.61039 x 10"2 m3/2 mol" m = 0.50925 dm 3/2 -mor 1/2 In these expressions, the first value is valid for basic SI units and the second for / in moles per cubic decimetre substituted into Eq. (1.3.24). Equation (1.3.24) is a very rough approximation and does not involve the individual characteristics of ion k. It is valid for a uni-univalent electrolyte only up to an ionic strength of 10~3 mol dm" 3 (see also Fig. 1.8). In view of the definition of the mean activity coefficient and of the electroneutrality condition, v+z+= v_z_, the limiting law also has the form logy =^z + z_V7 (1.3.25) m3/2 moP 1/2 dm3/2 mol"1/2

where Ea,i and Ci are the activation energy and a tting parameter, respectively, for the SRG and DG. It is found that the SRG begins disappearing B15 K before Tg. In contrast to this thermal erasure of SRGs, it appears that in some LC systems, thermal treatment after SRG formation leads to an enhancement of the grating height (Kawatsuki et al., 2003; Stracke et al., 2000). In these cases, heating may enable motion and aggregation of chromophores. Thin lm con nement effects have also been observed. In particular, thin lms cause an increase in the erasing temperature, equivalent to an increase of the apparent Tg by as much as 50 K (Yager and Barrett, 2007). The molecular-scale dynamics (e.g., isomerization) are negligibly affected by con nement, whereas the large-scale mass transport becomes arrested within B150 nm of the substrate interface.

1.3.2 More rigorous Debye-Hiickel treatment of the activity coefficient A more rigorous approach requires integration of Eq. (1.3.13) not over the whole volume of the solution but over the effective volume after the volume of the central ion has been excluded, as this region is not accessible for the ionic atmosphere. Thus, integration is carried out from r = ay i.e. from the distance of closest approach, equal to the effective ion diameter, which is the smallest mean distance to which the centres of other ions can approach the central ion. This value varies for various electrolytes (Table 1.3). In this refined procedure the integration constant appearing in Eq. (1.3.13) attains the value kx = [zkel4ne{\ + KO)\ exp {KO) and the potential \pk = zke/4jt [r(l + Ka)]'1 exp [ic(a r)]. This expression can again be separated into the contribution of the isolated central ion ip k and the contribution of the ionic atmosphere tya. As a result of the principle of linear field superposition, these two quantities can be added algebraically. The contribution of the

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Several mechanisms have been described to account for the microscopic origin of the driving force in azobenzene optical patterning. Arguments have appealed to thermal gradients, diffusion considerations, isomerization-induced pressure gradients, and interactions between azo dipoles and the electric eld of the incident light. Considering the large body of experimental observations, it is perhaps surprising that the issue of mechanism has not yet been settled. At present, no mechanism appears to provide an entirely complete and satisfactory explanation consistent with all known observations. However, viscoelastic modeling of the process has been quite successful, correctly reproducing nearly all experimentally observed surface patterns, without directly describing the microscopic nature of the driving force. Fluid mechanics models provided suitable agreement with observations (Barrett et al., 1998) and were later extended to take into account a depth dependence and a velocity distribution in the lm (Fukuda et al., 2000b; Sumaru et al., 1999), which reproduces the thickness dependence of SRG