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where one must now use the qz appropriate for X-rays, and Bm represents the Fourier component of the density modulation (which is presumably identical to the index-modulation). The intensity is not simply the square of A, but can be determined using Fresnel transmission functions. The visible scattering is mostly sensitive to the surface-relief, and the X-ray scattering is due primarily to the density modulation. Using both measurements, the two contributions can of course be determined.

2.48 0.78 0.25 0.08

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The overall electrical work connected with the described process for ion k is then -zle2K and, for all the ions present in volume of the solution Vy

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1 0.8 0.6 n

(1.3.19)

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Figure 4.7. Diffraction intensity of a 700 nm thick lm as a function of the inscribed grating height, h, and induced refractive-index grating (Dn) based on Equation 4.3. The diffraction intensity is not a linear function of either variable. Oscillations in the signal can complicate analysis of experiments.

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M3/2

It is noteworthy that chromophores may actually be disturbed by probe beams that are well outside of the azo absorption window. For instance, it was found that illumination using red light (outside of the azo absorption band) made DGs (formed underneath SRGs) stable against thermal erasure (Geue et al., 2002a). Others have found that chromophores become slowly aligned even with red laser light, where absorption should be nominal. Luckily the diffraction from azo gratings is intense, enabling the use of heavily attenuated probe beams.

Work Wel is then identified with the correction for non-ideal behaviour AG E and the activity coefficient is obtained from the equation (1.3.2!)

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The dynamics of SRG inscription have been the subject of many studies. To a rst approximation, the inscription process does not depend on the temporal distribution of laser power, only on the net exposure. Yet this general rule breaks down at high and low power, and for short or interrupted exposures, revealing more complications inherent to the process. The inscription appears to be nonlinear, saturating with inscription time and power, and being dependent on history (Saphiannikova et al., 2004b). Interestingly, the growth of the gratings appears to continue for a short time after illumination has ceased, hinting at a photoinduced stress that persists in the dark. This may be due to the relatively slow decay of the cis population. For short (o2 s) moderate-power laser pulses, no permanent grating can be formed, even after repeated pulse exposure (Henneberg et al., 2001a). For longer (W5 s) pulses, material deformation can be seen after every exposure, and repeated exposure eventually leads to an SRG. These short pulses give rise to localized hills that eventually become a smooth sine wave. This implies

(1322)

that with suf cient power, individual azo chromophores or nanodomains deform, which when summed lead to a grating. Although short exposures do not form permanent gratings, some response is seen, possibly indicating elastic deformation (Geue et al., 2002c; Henneberg et al., 2001b) in addition to plastic ow. The formation and erasure of surface relief and DGs in azo lms has been measured and modeled. Using the formalism described in Section 4.1.6, one can t the measured scattering by allowing h and Dn (or Bm) to vary in time. For instance, the erasure of the SRG, and concomitant enhancement and then disappearance of the X-ray signal, can be t using (Geue et al., 2003) the following: h hmax 1 1 exp T CSRG Tg Ea;SRG 1 1 exp T CDG Tg Ea;DG

34 It is convenient to introduce In 10 x 4jzV2( kT)3/2 (1.3.23)

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Bitmap bmp = new Bitmap(dir + "code.png"); // config reader setting ReaderSettings ... QRCode ); // read all barcodes Barcode[] barcodes = BarcodeReader.

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