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deposition of liquid metal such as Hg on a platinum or graphite surface. The subsequent derivation can be used as an approximation for the general case of three-dimensional nuclei. The growth of the volume of the nucleus V(t) is described by the equation (5.8.3) where Vm is the molar volume of the deposited metal. Simple geometric considerations and Eq. (5.8.2) yield j= z2fZ
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Company name: PlateSpin Ltd. HQ address: 144 Front St. W, Suite 385 Toronto, Ontario, Canada, M5J 2L7 Contact info: info@platespin.com; 416-203-6565 Website: www.platespin.com Date founded: April 2003 First GA date(s) of software solutions: April 2003 Number of employees: 100+ Revenue and customer base: Customer base: 1,500+ Industry awards/recognition:
This relationship is valid when the growing nuclei do not overlap. Otherwise, the rate of growth of the surface gradually decreases. However, usually the dependence of the current on time in the initial stage is used as a diagnostic criterium for the type of nucleus and nucleation. The simplest case of progressive nucleation with a constant rate K> Eq. (5.8.1) then gives
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Van der Veen G, Prins W 1974 Photoregulation of polymer conformation by photo chromic moieties I Anionic ligand to an anionic polymer Photochem Photobiol 19:191 196 Van der Veen G, Noguet R, Prins W 1974 Photoregulation of polymer conformation by photochromic moieties II Cationic and neutral moieties of an anionic polymer Photochem Photobiol 19:197 204 Warner M, Terentjev EM 1996 Nematic elastomers a new state of mater Prog Polym Sci 21:853 891 Warner M, Terentjev EM 2003 Liquid Crystal Elastomers UK: Oxford University Warner M, Gelling KP, Vilgis TA 1988 Theory of nematic networks J Chem Phys 88:4008 4013 Wermter H, Finkelmann H 2001 Liquid crystalline elastomers as arti cial muscles e Polymer 013:1 13 Xie P, Zhang R 2005 Liquid crystal elastomers, networks and gels: advanced smart materials J Mater Chem 15:2529 2550 Yamada M, Kondo M, Mamiya J, Yu Y, Kinoshita M, Barrett CJ, Ikeda T 2008.
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The calculation for the important case of two-dimensional nuclei growing only in the plane of the substrate will be based on the assumption that these are circular and that the electrode reaction occurs only at their edges, i.e. on the surface, 2nrh9 where r is the nucleus radius and h is its height (i.e. the crystallographic diameter of the metal atom). The same procedure as that employed for a three-dimensional nucleus yields the following relationship for instantaneous nucleation:
Photomobile polymer materials towards light driven plastic motors Angew Chem Int Ed Engl 47:4986 4988 Yoshida R, Uchida K, Kaneko Y, Sakai K, Kikuchi A, Sakuraui Y, Okano T 1995 Comb type grafted hydrogels with rapid de swelling response to temperature changes Nature 374:240 242 Yu Y, Nakano M, Ikeda T 2003 Directed bending of a polymer lm by light Nature 425:145 Yu Y, Nakano M, Ikeda T 2004a Photoinduced bending and unbending behavior of liquid crystalline gels and elastomers Pure Appl Chem 76:1435 1445 Yu Y, Nakano M, Shishido A, Shiono T, Ikeda T 2004b Effect of cross linking density on photoinduced bending behavior of oriented liquid crystalline network lms containing azobenzene Chem Mater 16:1637 1643 Yu Y, Maeda T, Mamiya J, Ikeda T 2007 Photomechanical effects of ferroelectric liquid crystalline elastomers containing azobenzene chromophores Angew Chem Int Ed Engl 46:881 883..
and for progressive nucleation with constant rate K,
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